Publications

Probing Single Jumps of Surface Atoms

Author(s)
Gero Vogl, Marcel Sladecek, S. Dattagupta
Abstract

Jumps of single atoms can be followed on their time and space scale (nanoseconds and Angstroms) by applying nuclear resonance scattering of synchrotron radiation. Here we develop the theory for jump diffusion in two-dimensional systems. Two types of phenomena are noteworthy: apparent acceleration of the nuclear decay and relaxation of hyperfine interactions, in particular, electric quadrupole interactions. The latter effect becomes for the first time one of significance and well measurable due to the inherent anisotropy of the surface. We show how, by way of motional narrowing, to distinguish between the motion of the probe atom itself and the motion of adatoms.

Organisation(s)
Dynamics of Condensed Systems
External organisation(s)
Philips Austria, Indian Institute of Science
Journal
Physical Review Letters
Volume
99
No. of pages
4
ISSN
0031-9007
DOI
https://doi.org/10.1103/PhysRevLett.99.155902
Publication date
2007
Peer reviewed
Yes
Austrian Fields of Science 2012
103015 Condensed matter
Portal url
https://ucrisportal.univie.ac.at/en/publications/eb1e8769-b2fa-489f-9652-0c6bcfe8e7ec